Functionalization of Carborane via Carboryne Intermediates

Nonfiction, Science & Nature, Science, Chemistry, Physical & Theoretical, Organic
Cover of the book Functionalization of Carborane via Carboryne Intermediates by Da Zhao, Springer Singapore
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Author: Da Zhao ISBN: 9789811015694
Publisher: Springer Singapore Publication: June 4, 2016
Imprint: Springer Language: English
Author: Da Zhao
ISBN: 9789811015694
Publisher: Springer Singapore
Publication: June 4, 2016
Imprint: Springer
Language: English

This thesis focuses on the development of new methods of functionalizing carboranes using o-carboryne intermediates. Functional carboranes are now finding a broad range of applications, including organic synthesis, drug design, polymers, catalysis, metal−organic frameworks, electronic devices and more. However, the limited number of efficient synthetic methods for obtaining functional carborane materials has restricted their applications. The methodologies established in this thesis represent simple, yet powerful strategies to assemble previously inaccessible, useful complex molecules, which will also have a significant impact on future synthetic, cluster and materials chemistry. Moreover, it discusses the first method for the in situ generation of electrophilic boron radical using photocatalysis.  

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This thesis focuses on the development of new methods of functionalizing carboranes using o-carboryne intermediates. Functional carboranes are now finding a broad range of applications, including organic synthesis, drug design, polymers, catalysis, metal−organic frameworks, electronic devices and more. However, the limited number of efficient synthetic methods for obtaining functional carborane materials has restricted their applications. The methodologies established in this thesis represent simple, yet powerful strategies to assemble previously inaccessible, useful complex molecules, which will also have a significant impact on future synthetic, cluster and materials chemistry. Moreover, it discusses the first method for the in situ generation of electrophilic boron radical using photocatalysis.  

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