High- and Low-Valent tris-N-Heterocyclic Carbene Iron Complexes

A Study of Molecular and Electronic Structure

Nonfiction, Science & Nature, Science, Chemistry, Inorganic, Technical & Industrial
Cover of the book High- and Low-Valent tris-N-Heterocyclic Carbene Iron Complexes by Carola S. Vogel, Springer Berlin Heidelberg
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Author: Carola S. Vogel ISBN: 9783642272547
Publisher: Springer Berlin Heidelberg Publication: February 3, 2012
Imprint: Springer Language: English
Author: Carola S. Vogel
ISBN: 9783642272547
Publisher: Springer Berlin Heidelberg
Publication: February 3, 2012
Imprint: Springer
Language: English

Carola Vogel’s PhD thesis focuses on the synthesis, and structural and spectroscopic characterization of the first high valent iron nitride complexes. In her interdisciplinary and collaborative research Carola also describes the reactivity studies of a unique iron (V) nitride complex with water. These studies show that quantitative yields of ammonia are given at ambient conditions. High valent iron nitride and oxo species have been proposed as key intermediates in many bio-catalytic transformations, but until now these species have proven exceedingly challenging to isolate and study. Iron complexes in high oxidation states can thus serve as models for iron-containing enzymes to help us understand biological systems or aid our development of more efficient industrial catalysts.

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Carola Vogel’s PhD thesis focuses on the synthesis, and structural and spectroscopic characterization of the first high valent iron nitride complexes. In her interdisciplinary and collaborative research Carola also describes the reactivity studies of a unique iron (V) nitride complex with water. These studies show that quantitative yields of ammonia are given at ambient conditions. High valent iron nitride and oxo species have been proposed as key intermediates in many bio-catalytic transformations, but until now these species have proven exceedingly challenging to isolate and study. Iron complexes in high oxidation states can thus serve as models for iron-containing enzymes to help us understand biological systems or aid our development of more efficient industrial catalysts.

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